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Validation of the inverted adsorption structure for free-base tetraphenyl porphyrin on Cu(111)

P T P Ryan1, P L Lalaguna, F Haag

  • 1Diamond Light Source, Harwell Science and Innovation Campus, Didcot, OX11 0QX, UK. david.duncan@diamond.ac.uk.

Chemical Communications (Cambridge, England)
|March 3, 2020
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Cycloheptatriene is a neutral monocyclic unsaturated hydrocarbon that consists of an odd number of carbon atoms and an intervening sp3 carbon in the ring. The three double bonds in the ring correspond to 6 π electrons, which is a Huckel number, and therefore satisfies the criteria of 4n + 2 π electrons. However, the intervening sp3 carbon disrupts the continuous overlap of p orbitals. As a result, cycloheptatriene is not aromatic.
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