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Updated: Dec 25, 2025

An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser
Guanqun Zhou1,2,3, Franz-Josef Decker2, Yuantao Ding2
1Key Laboratory of Particle Acceleration Physics and Technology, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing, 100049, China.
Characterizing ultra-fast hard x-ray pulse coherence time is crucial for free-electron laser (FEL) research. A novel cross-correlation method using a phase shifter successfully measured a 174.7 attosecond coherence time.
Area of Science:
- Physics
- Materials Science
- X-ray Science
Background:
- Characterizing the coherence time of ultra-fast hard x-ray pulses from free-electron lasers (FELs) is a significant challenge.
- This temporal coherence critically impacts x-ray-matter interaction processes.
- Conventional optical autocorrelation methods are impractical for hard x-rays due to the absence of suitable mirrors.
Purpose of the Study:
- To experimentally demonstrate a novel method for measuring the coherence time of ultra-fast hard x-ray pulses.
- To provide a universal diagnostic tool for temporal coherence applicable to various FEL parameters.
Main Methods:
- Utilizing a phase shifter to control the cross-correlation between the x-ray pulse and microbunched electrons.
- Experimental demonstration at the Linac Coherent Light Source (LCLS) for 6.92 keV FEL pulses.
Main Results:
- Successfully measured a coherence time of 174.7 attoseconds for the FEL pulses.
- The developed method is independent of general machine parameters.
Conclusions:
- The novel cross-correlation technique offers a viable solution for characterizing FEL pulse coherence time.
- This method is applicable across a wide range of photon energies, brightness, repetition rates, and pulse durations.
- The technique provides critical diagnostics for temporal coherence in x-ray FELs.
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