MBene (MnB): a new type of 2D metallic ferromagnet with high Curie temperature

We extend the 2D MXene family into the boride world, namely, MBenes. High-throughput calculations screen twelve MBenes with excellent stability. Among them, 2D MnB MBene exhibits robust metallic ferromagnetism (∼3.2 μ_B per Mn atom) and high Curie temperature (345 K). After functionalization with the -F and -OH groups, the ferromagnetic ground state of 2D MnB is well preserved. The Curie temperature is increased to 405 and 600 K, respectively, providing a novel and feasible strategy to tailor the T_C of 2D magnetic materials.