Related Experiment Video
Updated: Dec 24, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Multi-frame interferometric imaging with a femtosecond stroboscopic pulse train for observing irreversible phenomena
Dmitro Martynowych1, David Veysset2, A A Maznev1
1Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA.
Abstract:
We describe a high-speed single-shot multi-frame interferometric imaging technique enabling multiple interferometric images with femtosecond exposure time over a 50 ns event window to be recorded, following a single laser-induced excitation event. The stroboscopic illumination of a framing camera is made possible through the use of a doubling cavity that produces a femtosecond pulse train that is synchronized to the gated exposure windows of the individual frames of the camera. The imaging system utilizes a Michelson interferometer to extract phase and ultimately displacement information. We demonstrate the method by monitoring laser-induced deformation and the propagation of high-amplitude acoustic waves in a silicon nitride membrane. The method is applicable to a wide range of fast irreversible phenomena such as crack branching, shock-induced material damage, cavitation, and dielectric breakdown.

