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Setting the photoelectron clock through molecular alignment.

Andrea Trabattoni1,2, Joss Wiese1,3, Umberto De Giovannini4

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Summary
This summary is machine-generated.

Strong laser fields interacting with aligned molecules reveal real-time electron dynamics. The molecule dictates electron emission timing and energy, impacting strong-field physics interpretations.

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Area of Science:

  • Atomic, Molecular, and Optical Physics
  • Strong-Field Physics
  • Quantum Dynamics

Background:

  • Strong laser fields enable high-resolution imaging of transient dynamics.
  • Understanding electron behavior in molecular systems is crucial for advanced physics.
  • Molecular alignment influences light-matter interactions.

Purpose of the Study:

  • To visualize real-time photoelectron dynamics during strong-field ionization of laser-aligned molecules.
  • To investigate the impact of molecular structure on electron emission and rescattering.
  • To establish a benchmark for molecular-frame strong-field physics.

Main Methods:

  • Utilizing strong laser fields to ionize laser-aligned molecules.
  • Simulating and analyzing photoelectron dynamics in real-time.
  • Examining photoelectron momentum distributions.

Main Results:

  • The molecule significantly influences strong-field dynamics, controlling electron emission timing and rescattering energy.
  • A real-time picture of photoelectron dynamics under combined laser and molecular fields was achieved.
  • Molecular-frame photoelectron momentum distributions encode time-energy relationships.

Conclusions:

  • Molecular structure acts as a 'clock' for electron emission in strong-field interactions.
  • This work provides critical insights for interpreting self-diffraction experiments.
  • The findings pave the way for real-time probing of molecular potentials and electron transport.