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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Research Progresses of Garnet-Type Solid Electrolytes for Developing All-Solid-State Li Batteries.

Abin Kim1, Seungjun Woo1, Minseok Kang1

  • 1Department of Materials Science and Engineering, Pohang University of Science and Technology (POSTECH), Gyeongbuk, South Korea.

Frontiers in Chemistry
|July 17, 2020
PubMed
Summary

All-solid-state batteries (ASSBs) using oxide solid electrolytes offer enhanced safety and energy density. This review focuses on garnet-type electrolytes and addresses challenges like interfacial resistance and lithium dendrite growth for practical ASSB applications.

Keywords:
Li ion batteriesall-solid-state-batteriesbeyond Li-ion batteriesgarnet-type electrolytesolid electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) with oxide-based solid electrolytes (SEs) are promising for high-energy, safe energy storage, surpassing traditional Li-ion batteries (LIBs).
  • Practical application of ASSBs is limited by high interfacial resistance and challenges associated with using lithium metal anodes.
  • Oxide-based SEs are crucial for advancing battery technology due to their potential for improved safety and energy density.

Purpose of the Study:

  • To review recent advancements in oxide-based SEs for ASSBs, specifically focusing on their compatibility with lithium metal anodes.
  • To highlight the potential of garnet-type solid electrolytes (Li7La3Zr2O12) due to their high ionic conductivity, chemical stability, and wide electrochemical window.
  • To discuss lithium dendrite formation and its impact on critical current density (CCD) in oxide-based SEs.

Main Methods:

  • Literature review of recent research on oxide-based solid electrolytes for ASSBs.
  • Focus on garnet-type Li7La3Zr2O12 as a representative and promising solid electrolyte material.
  • Analysis of lithium dendrite behavior and its correlation with critical current density (CCD) in solid electrolytes.

Main Results:

  • Garnet-type solid electrolytes exhibit excellent ionic conductivity, chemical stability with lithium metal, and a broad electrochemical potential window.
  • Understanding lithium dendrite growth mechanisms and their relationship with critical current density is key to enabling stable lithium metal cycling.
  • Interfacial resistance remains a significant hurdle for the practical implementation of composite electrodes and Li metal anodes in ASSBs.

Conclusions:

  • Garnet-type solid electrolytes are highly promising for developing safe and high-performance ASSBs.
  • Further research is needed to mitigate interfacial resistance and control lithium dendrite growth for commercial viability.
  • ASSBs hold significant potential for next-generation energy storage solutions if current challenges are effectively addressed.