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Updated: Dec 14, 2025

Extraction and Characterization of Surfactants from Atmospheric Aerosols
Published on: April 21, 2017
Exploring aerosols near clouds with high-spatial-resolution aircraft remote sensing during SEAC4RS
Robert S Spencer1,2, Robert C Levy2, Lorraine A Remer3
1Science Systems and Applications, Inc, Lanham, Maryland, USA.
High-resolution satellite data reveals aerosols near clouds significantly enhance aerosol optical depth (AOD). This enhancement is primarily caused by 3D radiative interactions between clouds and the surrounding atmosphere, not just aerosol swelling.
Area of Science:
- Atmospheric Science
- Remote Sensing
- Climate Science
Background:
- Aerosols significantly influence Earth's climate system.
- Satellite-borne Moderate-resolution Imaging Spectroradiometer (MODIS) Dark Target (DT) algorithm retrieves aerosol optical depth (AOD) in cloud-free conditions.
- MODIS resolution is insufficient for studying aerosols near clouds.
Purpose of the Study:
- To investigate aerosol variability within cloud systems using high-resolution data.
- To analyze the causes of enhanced AOD observed near clouds.
Main Methods:
- Porting the Dark Target (DT) algorithm to the enhanced-MODIS Airborne Simulator (eMAS) for high-resolution (~50 m pixels) retrievals.
- Utilizing data from the SEAC4RS campaign (2013) including eMAS, Cloud Physics Lidar (CPL), MODIS, and AERONET observations.
- Defining spatial metrics to differentiate near-cloud and far-from-cloud environments.
Main Results:
- High-resolution eMAS retrievals showed enhanced AOD within 6 km of clouds, even with aggressive cloud screening.
- Cloud masking was robust; thin cirrus had minimal impact on retrieved AOD.
- Observed AOD enhancement is partly explained by aerosol swelling in clear-cloud transition zones.
Conclusions:
- Three-dimensional radiative interactions between clouds and the surrounding clear air are the primary driver of enhanced AOD near clouds.
- High-resolution airborne remote sensing is crucial for understanding near-cloud aerosol properties.
- Findings improve the understanding of aerosol-cloud interactions and their climate implications.
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