Unraveling the Origin of Tribomagnetization in Ferromagnetic Materials

Tribomagnetization, a natural phenomenon known for decades, has many engineering applications today. However, its intrinsic origin remains controversial and the mechanistic-based model has not yet been developed to predict the tribomagnetization behavior. In this work, the origin of tribomagnetization is investigated via both the experimental and modeling approaches. For the first time, the expansion of surface plastic deformation to the subsurface layer (i.e., dislocation strain gradient) is characterized in conjunction with the tribological behavior of the interface. By performing the reciprocating sliding experiment in a pin-on-block contact configuration, the tribomagnetization evolution in different wear regimes is followed, the geometrically necessary dislocations (GNDs) developed in the subsurface are measured, and the formation of characteristic magnetic domains is revealed. A tribomagnetization model is proposed on the basis of the sliding-induced plastic deformation mechanism with GNDs, bringing the missing link with classical tribology and ferromagnetism. The model reveals that the surface plastic strain and width of a wear scar are two crucial factors in determining the surface magnetic field changes. We believe that the tribomagnetization originates from the magnetic distortion accompanied by the progression of GNDs in the subsurface. Our hypothesis is supported by the good agreement between the model prediction and experimental observation.