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Updated: Nov 29, 2025

Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Published on: August 12, 2013

Printable, high-performance solid-state electrolyte films.

Weiwei Ping¹, Chengwei Wang¹, Ruiliu Wang¹

¹Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.

Science Advances

|November 19, 2020

Summary

This summary is machine-generated.

Researchers developed a rapid printing and sintering method to create high-performance ceramic solid-state electrolyte (SSE) films. This technique significantly boosts ionic conductivity and fabrication speed for safer, more efficient solid-state batteries.

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Last Updated: Nov 29, 2025

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Published on: August 12, 2013

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Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Published on: November 11, 2013

Area of Science:

Materials Science
Electrochemistry
Solid-State Chemistry

Background:

Current ceramic solid-state electrolyte (SSE) films suffer from low ionic conductivity due to amorphous structures or lithium loss.
Existing fabrication methods are time-consuming and limit the development of high-performance solid-state batteries.

Purpose of the Study:

To develop a novel, rapid fabrication process for high-performance ceramic SSE films.
To enhance ionic conductivity and reduce fabrication time compared to conventional methods.
To demonstrate the applicability of the fabricated SSEs in solid-state batteries.

Main Methods:

A solution-based printing process followed by rapid (~3 seconds) high-temperature (~1500°C) reactive sintering was employed.
The process allows for layer-by-layer fabrication of multilayer structures without cross-contamination.
Fabrication time from precursor to final product is approximately 5 minutes.

Main Results:

The fabricated ceramic SSE films exhibit a dense, uniform structure.
Superior ionic conductivity of up to 1 mS/cm was achieved.
The fabrication process is 10 to 100 times faster than conventional SSE syntheses.
A printed solid-state battery demonstrated conformal interfaces and excellent cycling stability.

Conclusions:

The printing and rapid sintering technique offers a fast and efficient route to high-performance ceramic SSEs.
This method overcomes limitations of current SSE fabrication, enabling improved solid-state batteries.
The technique is versatile and can be applied to other thin-film SSEs for advanced device applications.