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Updated: Nov 26, 2025

Fabrication of Three-Dimensional Graphene-Based Polyhedrons via Origami-Like Self-Folding
Published on: September 23, 2018
Layer-by-layer assembly into bulk-like g-C3N4via artificial manipulation of electrostatic forces
Yan Wang1, Guangshe Li, Yuelan Zhang
1State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, P. R. China. guangshe@jlu.edu.cn lipingli@jlu.edu.cn.
Abstract:
For the first time, bulk-like g-C3N4 was achieved through initiating layer-by-layer assembly, which involves the important process of artificially manipulating protonated and oxygen doped g-C3N4 nanosheets. When acting as a photocatalyst under UV-visible light irradiation, bulk-like g-C3N4 exhibited an excellent photocatalytic H2 production rate of 1538 μmol h-1 g-1, about 8 times higher than that of the bulk g-C3N4 counterpart.
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