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Li7La3Zr2O12 Garnet Solid Polymer Electrolyte for Highly Stable All-Solid-State Batteries.

Quoc Hung Nguyen1, Van Tung Luu1, Hoang Long Nguyen1

  • 1Department of Energy Systems Engineering, Soonchunhyang University, Asan-si, South Korea.

Frontiers in Chemistry
|February 4, 2021
PubMed
Summary
This summary is machine-generated.

Researchers developed a composite electrolyte using cubic garnet oxide (LLZO) and ionic liquid to enhance all-solid-state batteries. This novel material improves ionic conductivity and suppresses lithium dendrite growth for safer, high-performance energy storage.

Keywords:
all-solid-state batteriescubic garnet LLZOionic-liquidlithium dendrite growth suppressionsolid polymer electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries offer enhanced safety and stability over traditional lithium-ion batteries.
  • Solid polymer electrolytes face challenges with low ionic conductivity and lithium metal compatibility.
  • Lithium dendrite formation remains a critical issue hindering the performance and safety of solid-state batteries.

Purpose of the Study:

  • To develop a composite electrolyte membrane combining cubic garnet oxide (Li7La3Zr2O12 - LLZO) and ionic liquid with a polymer electrolyte.
  • To enhance ionic conductivity and suppress lithium dendrite growth in all-solid-state batteries.
  • To evaluate the electrochemical performance of the composite electrolyte in a full cell configuration.

Main Methods:

  • Fabrication of a composite electrolyte membrane incorporating LLZO, ionic liquid, and polymer electrolyte.
  • Characterization of ionic conductivity at elevated temperatures.
  • Symmetric lithium stripping/plating tests to assess lithium dendrite suppression.
  • Fabrication and testing of a full cell using lithium iron phosphate cathode and the composite electrolyte.

Main Results:

  • The composite electrolyte membrane exhibited high ionic conductivity at elevated temperatures.
  • LLZO effectively suppressed lithium dendrite growth, evidenced by small polarization voltages in stripping/plating tests.
  • The full cell achieved a specific capacity of 137.4 mAh g⁻¹ and 98.47% capacity retention after 100 cycles at 60°C.
  • High specific discharge capacities of 137 and 100.8 mAh g⁻¹ were recorded at 100 and 200 mA g⁻¹, respectively.

Conclusions:

  • The developed composite electrolyte demonstrates significant potential for improving all-solid-state battery performance.
  • The combination of LLZO and ionic liquid in a polymer matrix effectively addresses key challenges in solid-state battery technology.
  • This approach offers a viable pathway towards safer and more efficient high-performance energy storage solutions.