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Related Experiment Video

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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Ultra-high throughput manufacturing method for composite solid-state electrolytes.

Paul Baade1, Vanessa Wood1

  • 1Department of Information Technology and Electrical Engineering, Materials and Device Engineering Group, ETH Zurich, 8092 Zürich, Switzerland.

Iscience
|February 4, 2021
PubMed
Summary

Manufacturing solid-state batteries affordably is key for safer, high-energy lithium ion batteries. Curtain coating enables high-speed, roll-to-roll production of thin, uniform composite solid-state electrolytes, compatible with current manufacturing.

Keywords:
Electrochemical Energy StorageElectrochemistryEnergy MaterialsEngineeringMechanical Engineering

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Area of Science:

  • Materials Science
  • Chemical Engineering
  • Electrochemistry

Background:

  • Solid-state electrolytes offer enhanced safety and energy density for lithium ion batteries compared to liquid organic electrolytes.
  • Scalable and cost-effective manufacturing remains a significant challenge for widespread adoption of solid-state battery technology.

Purpose of the Study:

  • To introduce and validate curtain coating as a viable manufacturing method for composite solid-state electrolytes.
  • To demonstrate the compatibility of curtain coating with existing roll-to-roll manufacturing processes for lithium ion batteries.

Main Methods:

  • Development and application of a curtain coating technique for depositing composite solid-state electrolyte films.
  • Integration of the curtain coating process into a roll-to-roll manufacturing setup.
  • Characterization of electrolyte film uniformity and thickness.

Main Results:

  • Successful demonstration of curtain coating for manufacturing composite solid-state electrolytes at high web-speeds exceeding 80 m/min.
  • Production of uniform electrolyte films with thicknesses below 15 micrometers.
  • Compatibility of the proposed method with existing lithium-ion battery manufacturing infrastructure.

Conclusions:

  • Curtain coating presents a scalable, high-throughput solution for manufacturing composite solid-state electrolytes.
  • This method addresses the critical need for cost-effective and large-scale production of solid-state batteries.
  • The technology facilitates the commercial viability of safer and more energy-dense lithium ion batteries.