Heavy metal(loid)s in sewage sludge in China: concentrations and spatial-temporal variations

Sewage sludge (SS) production in China has increased rapidly, accompanying the fast expansion of its sewage treatment capacity. Heavy metals (HMs) in SS have been a great concern, hampering the utilization and disposal of SS. In this study, heavy metal (HM) contents in SS from throughout China were determined. The median values of HMs in SS decreased in the order Zn > Cu > Cr > Pb > Ni > As > Hg > Cd. The general attainment rates of HMs in SS are satisfying (> 90%). Combining the present data with those obtained from references, spatial distributions and temporal trends of HMs in SS were analyzed. Depending on the specific HM element, the spatial variation trend might be decreasing trends from south to north and from east to west of China. The element-specific hot spots of SS with relatively high HM contents were identified. Analysis of the historical data in different time intervals reviewed obvious decreasing trends in HM contents of SS in China, indicating the well implementation of more and more stringent environmental regulations.