Meteorology governs the variation of Delhi's high particulate-bound chloride levels

A significant number of past studies have reported Delhi to witness some of the highest levels of particulate-bound chloride compared to anywhere else in the world. The present study employs long-term, highly time-resolved chloride measurements at the IIT Delhi campus from February 2020 to April 2021. The present work sheds light on the dependence of high chloride levels in Delhi on the winds from the northwest direction. The study makes use of linear regression models and stepped linear models to quantify the role of meteorological variables in driving the seasonal variation of chloride in Delhi. The results indicate that ∼85-88% of the variation in chloride concentration observed in Delhi can be attributed to meteorological parameters, mainly temperature (T), relative humidity (RH), and percentage of wind incoming from the northwest (%NW). The results also suggest that the primary chloride emissions remain relatively consistent year-round, and are regionally transported from Delhi's northwest. The results of this study provide valuable insights in understanding the nature of the sources and the variability associated with the chloride levels in Delhi and thus provide a basis for future emission control strategies.