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Quantifying Spin-Mixed States in Ferromagnets
Justin M Shaw1, Ronny Knut2, Abigail Armstrong3
1Quantum Electromagnetics Division, National Institute of Standards and Technology, Boulder, Colorado 80305, USA.
Abstract:
We quantify the presence of spin-mixed states in ferromagnetic 3D transition metals by precise measurement of the orbital moment. While central to phenomena such as Elliot-Yafet scattering, quantification of the spin-mixing parameter has hitherto been confined to theoretical calculations. We demonstrate that this information is also available by experimental means. Comparison of ferromagnetic resonance spectroscopy with x-ray magnetic circular dichroism results show that Kittel's original derivation of the spectroscopic g factor requires modification, to include spin mixing of valence band states. Our results are supported by ab initio relativistic electronic structure theory.
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