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Open quantum dynamics theory for a complex subenvironment system with a quantum thermostat: Application to a spin
Kiyoto Nakamura1, Yoshitaka Tanimura1
1Department of Chemistry, Graduate School of Science, Kyoto University, Sakyoku, Kyoto 606-8502, Japan.
The Journal of Chemical Physics
|January 1, 2022
Summary
This study introduces a quantum thermostat model for simulating complex environments, revealing that a two-level system (TLS) decoheres even with extreme anisotropy in its subenvironment.
Area of Science:
- Condensed matter physics
- Quantum dynamics
- Quantum information science
Background:
- Complex environments significantly influence dynamics in condensed phases.
- Simulating these environments is challenging due to numerous degrees of freedom.
- Existing models struggle to capture non-local, non-Gaussian noise characteristic of complex subenvironments.
Purpose of the Study:
- To develop and validate a novel quantum thermostat model for simulating quantum dynamics in complex environments.
- To investigate the impact of subenvironment properties, including quantum phase transitions, on a two-level system (TLS).
- To analyze decoherence and relaxation processes of a TLS interacting with a spin chain subenvironment.
Main Methods:
- A hybrid model combining a detailed subenvironment (1D XXZ spin chain) with a harmonic bath quantum thermostat.
- Simulation of a two-level system (TLS) dynamics interacting with the subenvironment.
- Utilizing hierarchical Schrödinger equations of motion for time-irreversible simulations at arbitrary temperatures.
Main Results:
- Observed decoherence of the TLS at finite temperatures, even under extreme spin anisotropy conditions.
- Demonstrated that subenvironment noise is spatially non-local and non-Gaussian, defying simple fluctuation-dissipation theorem characterization.
- Found complex changes in TLS population-relaxation dynamics correlating with spin anisotropy and magnetic ordering (ferromagnetic/antiferromagnetic).
Conclusions:
- The quantum thermostat model provides a viable approach for simulating quantum dynamics in complex, many-body environments.
- Subenvironment properties, particularly quantum phase transitions, critically affect TLS dynamics like decoherence and relaxation.
- The model captures intricate environmental effects beyond standard approximations, offering insights into quantum processes in realistic systems.
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