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Updated: Oct 4, 2025

Author Spotlight: Experimental Approaches for the Synthesis of Low-Valent Metal-Organic Frameworks from Multitopic Phosphine Linkers

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Proton Conductive Lanthanide-Based Metal-Organic Frameworks: Synthesis Strategies, Structural Features, and Recent

Hui-Min Ren¹, Hong-Wei Wang¹, Yuan-Fan Jiang¹

¹College of Chemistry and Green Catalysis Center, Zhengzhou University, 450001, Henan, PR China.

Topics in Current Chemistry (Cham)

|February 4, 2022

Summary

Lanthanide-based metal-organic frameworks (Ln-MOFs) show promise as advanced proton conductive materials for applications like proton exchange membrane fuel cells. Their unique structure offers enhanced water stability and high proton conductivity, addressing key challenges in material development.

Keywords:

Lanthanide MOFs Mechanism Progress Proton conduction

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Area of Science:

Materials Science
Chemistry
Electrochemistry

Background:

Proton conductive materials are crucial for proton exchange membrane fuel cells (PEMFCs), molecular sieves, and biochemistry.
Developing next-generation proton conductive materials with high conductivity and water stability, such as crystalline metal-organic frameworks (MOFs), presents significant challenges.

Purpose of the Study:

This review consolidates the latest advancements in proton conductive lanthanide-based MOFs (Ln-MOFs).
It explores synthesis strategies, structural characteristics, proton conductivity, conductive mechanisms, and applications of Ln-MOFs.
The review aims to identify design principles and future development directions for Ln-MOFs by analyzing structure-property relationships.

Main Methods:

Literature review of recent research on proton conductive Ln-MOFs.
Analysis of synthesis strategies and structural features of Ln-MOFs.
Evaluation of proton conductivity, mechanisms, and stability data.

Main Results:

Ln-MOFs exhibit superior water stability compared to transition metal analogues due to lanthanide properties.
Ln-MOFs demonstrate significant potential for high proton conductivity.
Structure-property relationships offer insights into designing advanced Ln-MOFs.

Conclusions:

Ln-MOFs are highly promising candidates for next-generation proton conductive materials.
Further research into their synthesis and structural design can optimize their performance for applications like PEMFCs.
Understanding structure-property correlations is key to unlocking the full potential of Ln-MOFs.