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Disentangling Coexisting Structural Order Through Phase Lock-In Analysis of Atomic-Resolution STEM Data.

Berit H Goodge1, Ismail El Baggari2, Seung Sae Hong3,4

  • 1School of Applied and Engineering Physics, Cornell University, Ithaca, NY14853, USA.

Microscopy and Microanalysis : the Official Journal of Microscopy Society of America, Microbeam Analysis Society, Microscopical Society of Canada
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PubMed
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This study introduces a new phase analysis technique for atomic-resolution STEM imaging. It reveals complex structural details and multiple order parameters in quantum materials, offering deeper insights into material properties.

Keywords:
atomic resolution STEMgeometric phase analysisheterogeneityquantum materialssuperlattice

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Nanotechnology

Background:

  • Atomic-resolution STEM imaging provides amplitude and geometric phase information.
  • Geometric Phase Analysis (GPA) typically maps elastic strain.
  • Crystalline lattices contain local variations and heterogeneities.

Purpose of the Study:

  • To demonstrate an alternative phase demodulation technique for STEM imaging.
  • To reveal complex structural phenomena in correlated quantum materials.
  • To extract multiple order parameters and analyze their interplay.

Main Methods:

  • Developed a novel phase demodulation technique.
  • Applied the technique to atomic-resolution STEM images.
  • Extended phase analysis to Fourier components encoding lattice modulations.

Main Results:

  • Successfully extracted detailed information on structural order and disorder, including dislocations and defects.
  • Revealed the behavior of multiple distinct order parameters within a single image.
  • Visualized the spatial interplay between various structural orders in novel materials.

Conclusions:

  • The phase lock-in approach provides insights into crystalline heterogeneity and emergent order parameters like antipolar displacements.
  • This method enables vivid visualizations of complex structural phenomena over large fields of view.
  • The technique offers a powerful tool for studying novel quantum materials.