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Charge transport in the spatially correlated exponential random energy landscape: effect of the nonpositive

Sergey Novikov¹

¹A.N. Frumkin Institute of Physical Chemistry and Electrochemistry, Leninsky Prosp. 31, Moscow 119071, Russia. novikov@elchem.ac.ru.

Physical Chemistry Chemical Physics : PCCP

|April 7, 2022

Abstract:

Charge transport in amorphous semiconductors having spatially correlated exponential density of states (DOS) has been considered for the arbitrary behavior of the correlation function of random energies. Average carrier velocity is exactly calculated for the quasi-equilibrium (nondispersive) transport regime. For the symmetric exponential DOS with exponential tails for low and high energies and nonpositive correlation function the temperature of the transition to the dispersive transport regime depends on correlation properties and becomes greater than the traditional estimation based on the DOS decay energy kT = U₀. Another new feature of the transport in the landscape having nonpositive correlation function is the decrease of the mobility with the field in the low field region and development of the universal mobility field dependence for stronger fields.

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