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Ionic Bonding and Electron Transfer02:48

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Ions are atoms or molecules bearing an electrical charge. A cation (a positive ion) forms when a neutral atom loses one or more electrons from its valence shell, and an anion (a negative ion) forms when a neutral atom gains one or more electrons in its valence shell. Compounds composed of ions are called ionic compounds (or salts), and their constituent ions are held together by ionic bonds: electrostatic forces of attraction between oppositely charged cations and anions. 
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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High-Content Lithium Aluminum Titanium Phosphate-Based Composite Solid Electrolyte with Poly(ionic liquid) Binder.

Fujie Yang1, Qingfeng Liu1, Wenfei Xie1

  • 1GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Polymers
|April 12, 2022
PubMed
Summary
This summary is machine-generated.

Flexible composite solid electrolytes using lithium aluminum titanium phosphate (LATP) and poly(ionic liquid) binders offer enhanced ionic conductivity and mechanical strength for next-generation electronics.

Keywords:
hardnessionic conductivitylithium aluminum titanium phosphatepoly(ionic liquid)solid-state electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Science

Background:

  • Solid electrolytes are crucial for safe and machinable flexible electronics.
  • Traditional solid electrolytes often lack sufficient ionic conductivity or flexibility.

Purpose of the Study:

  • To develop a composite solid electrolyte (CSE) with improved flexibility and ionic conductivity.
  • To investigate the effect of a poly(ionic liquid) binder on the properties of lithium aluminum titanium phosphate (LATP) based electrolytes.

Main Methods:

  • Fabrication of CSEs using LATP as a ceramic matrix and modified poly(ionic liquid) as a binder.
  • Characterization of ionic conductivity and Vickers hardness of the CSEs.
  • Optimization of LATP content for maximum performance.

Main Results:

  • The addition of poly(ionic liquid) binder significantly enhanced ionic conductivity and flexibility.
  • The CSE with 50 wt.% LATP achieved the highest ionic conductivity of 1.2 × 10-3 S·cm-1, an order of magnitude higher than pristine LATP.
  • The CSE exhibited a Vickers hardness of 0.9 ± 0.1 gf/mm2 at 50 wt.% LATP content.

Conclusions:

  • Composite solid electrolytes incorporating poly(ionic liquid) binders offer a promising pathway for advanced flexible electronic devices.
  • The developed CSE demonstrates a favorable balance of ionic conductivity and mechanical robustness.
  • This material design addresses key challenges in solid-state electrolyte development for next-generation batteries and electronics.