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Efficient All-Polymer Solar Cells with Sequentially Processed Active Layers.

Chaoyue Zhao1, Hui Huang1, Lihong Wang1

  • 1College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China.

Polymers
|May 28, 2022
PubMed
Summary
This summary is machine-generated.

Sequential processing (SqP) improves electron mobility in all-polymer solar cells (all-PSCs), enhancing charge transport and device performance. This method offers comparable results to blend-casting (BC) by boosting fill factor and compensating for current loss.

Keywords:
all-polymer solar cellspolymerized small-molecule acceptorssequential processing

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Area of Science:

  • Materials Science
  • Organic Electronics
  • Photovoltaics

Background:

  • All-polymer solar cells (all-PSCs) are promising for flexible and low-cost photovoltaics.
  • Low electron mobility in polymerized small-molecule acceptor (PSMA)-based all-PSCs hinders performance.
  • Current processing methods like blend-casting (BC) face limitations in optimizing charge transport.

Purpose of the Study:

  • To investigate the sequential processing (SqP) method for enhancing electron mobility in all-PSCs.
  • To analyze the impact of SqP on charge carrier transport and device performance.
  • To understand the relationship between electron mobility and device characteristics using depth-dependent analysis.

Main Methods:

  • Application of the sequential processing (SqP) method to PM6/PY-IT all-PSCs.
  • Comparison of SqP with the conventional blend-casting (BC) method.
  • Film-depth-dependent light absorption spectroscopy to analyze vertical charge dynamics.

Main Results:

  • SqP significantly boosts electron mobility and improves charge carrier balance in all-PSCs.
  • The SqP method increases the fill factor (FF) and compensates for short-circuit current loss.
  • Overall device performance achieved with SqP is comparable to that of BC devices.

Conclusions:

  • Sequential processing is an effective strategy to overcome low electron mobility in PSMA-based all-PSCs.
  • Enhanced electron mobility via SqP leads to improved charge transport and device efficiency.
  • SqP offers a viable alternative processing technique for advancing all-polymer solar cell technology.