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Recent Progress in Graphene-Based Electrocatalysts for Hydrogen Evolution Reaction.

Xupeng Qin1, Oluwafunmilola Ola2, Jianyong Zhao1

  • 1Guangxi Institute Fullerene Technology (GIFT), Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education, School of Resources, Environment and Materials, Guangxi University, Nanning 530004, China.

Nanomaterials (Basel, Switzerland)
|June 10, 2022
PubMed
Summary
This summary is machine-generated.

Graphene-based catalysts are promising for efficient hydrogen production via water splitting. This review covers synthesis, applications, and strategies for enhancing graphene electrocatalysts for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER).

Keywords:
3D structureelectrocatalysisgrapheneheteroatom-doped graphenehydrogen evolution reaction

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Renewable Energy

Background:

  • Hydrogen is a key renewable energy carrier for future demands.
  • Graphene and its derivatives offer advantages like high conductivity and eco-friendliness for electrocatalysis.
  • Electrocatalytic water splitting is crucial for sustainable hydrogen production.

Purpose of the Study:

  • To review recent advances in graphene-based electrocatalysts for the hydrogen evolution reaction (HER).
  • To discuss synthesis strategies and applications of various graphene-based catalysts.
  • To explore bifunctional electrocatalysts for both HER and oxygen evolution reaction (OER) in water electrolysis.

Main Methods:

  • Review of literature on synthesis and application of graphene-based electrocatalysts.
  • Highlighting powder-based and 3D self-supporting catalysts.
  • Discussion of defect engineering and heteroatom doping strategies.

Main Results:

  • Graphene-based materials, including quantum dots and doped/undoped heteroatom graphene, show significant promise for HER.
  • Strategies for tuning structural properties and performance of HER electrocatalysts are discussed.
  • Multi-doped graphene-based electrocatalysts are effective for bifunctional HER and OER.

Conclusions:

  • Graphene-based electrocatalysts are vital for efficient and sustainable hydrogen production.
  • Rational design and synthesis strategies are identified for high-performance catalysts.
  • Further development of graphene-based materials will advance green energy applications.