Preparation of Highly Stable and Electrochemically Active Three-dimensional Interconnected Graphene Frameworks from...

Over the past few years, the environmentally friendly synthesis of nanomaterials, including graphene using green chemistry, has attracted tremendous attention due to its easy handling, low cost, and biocompatibility. Here we demonstrate a facile and efficient green synthesis route for producing highly stable and electrochemically active three-dimensional interconnected graphene frameworks (3DIGF) from jute sticks. Initially, jute sticks derived three-dimensional amorphous activated carbon nanosheets (3DAACNs) were prepared at low temperatures (i. e., 850 °C) in an inert environment. The resultant 3DAACNs were then heat treated at a high temperature (i. e., 2700 °C) under an inert environment, resulting in 3DIGF. The prepared carbonaceous materials were fully characterized, and various experimental techniques confirmed the preparation of 3DIGF. The prepared 3DIGF shows a highly stable nature in thermal and chemical environments and demonstrates a highly dynamic nature for the electrooxidation of sulfide. This study could be considered a vital contribution towards the economic and simple approach for preparing 3DIGF from biomass.