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Developments in Surface/Interface Engineering of Ni-Rich Layered Cathode Materials.

Xiaomei Wang1, Xiaopeng Ruan1, Cheng-Feng Du2

  • 1State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal Materials, Northwestern Polytechnical University Xi'an, Shaanxi, 710072, P. R. China.

Chemical Record (New York, N.Y.)
|June 22, 2022
PubMed
Summary
This summary is machine-generated.

Surface engineering enhances Ni-rich cathodes for stable, high-energy lithium-ion batteries (LIBs). This review details methods to improve cathode-electrolyte interface stability and performance for reliable energy storage.

Keywords:
Failure mechanismsLithium-ion batteriesNi-rich cathode materialSurface engineering

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Ni-rich layered cathodes offer high energy density for lithium-ion batteries (LIBs).
  • Poor stability and cathode-electrolyte interface (CEI) reactions limit their practical application.
  • Surface and interface modifications are crucial for enhancing stability and performance.

Purpose of the Study:

  • To provide a comprehensive review of surface engineering strategies for Ni-rich cathode materials.
  • To summarize failure mechanisms and discuss existing surface modification techniques.
  • To elaborate on recent breakthroughs and future outlook for Ni-rich cathodes.

Main Methods:

  • Literature review and analysis of surface modification techniques for Ni-rich cathodes.
  • Categorization of surface coatings and modification strategies.
  • Discussion of functionalities for structural protection and performance enhancement.

Main Results:

  • Failure mechanisms during synthesis and operation of Ni-rich cathodes are summarized.
  • Various surface modification techniques, including coatings, are discussed and compared.
  • Recent advancements in surface engineering demonstrate improved structural integrity and electrochemical performance.

Conclusions:

  • Surface engineering is essential for overcoming the stability limitations of Ni-rich cathodes.
  • Optimized surface modifications can significantly enhance the performance and reliability of LIBs.
  • Further research is needed to address challenges and unlock the full potential of these materials.