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Updated: Aug 25, 2025

Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Cross-polarized common-path temporal interferometry for high-sensitivity strong-field ionization measurements.
A new interferometer precisely measures plasma density, crucial for laser-plasma interactions and atmospheric studies. Experiments with noble gases and hydrogen validate theoretical models like ADK and PPT for ionization pathways.
Area of Science:
- Plasma Physics
- Laser-Induced Phenomena
- Quantum Optics
Background:
- Accurate plasma density measurements are vital for understanding laser-matter interactions.
- Applications include strong-field physics, laser pulse propagation, and Lidar technology.
- Existing methods often lack the required sensitivity for low-density plasmas.
Purpose of the Study:
- To develop a highly sensitive interferometer for absolute plasma density measurements.
- To investigate strong-field ionization yields in noble gases using different laser polarizations.
- To study photoionization and photodissociation of molecular hydrogen.
Main Methods:
- A cross-polarized common-path temporal interferometer with balanced detection was employed.
- Measurements utilized 800 nm, 55 fs laser pulses for noble gas ionization studies.
- Experimental data were compared against Ammosov-Delone-Krainov (ADK) and Perelomov-Popov-Terent'ev (PPT) theoretical models.
Main Results:
- The interferometer achieved a sensitivity of ~0.6 mrad, enabling density-length product measurements of ~2.6 x 10^13 cm^-2.
- Measured phase changes for noble gases aligned with ADK theory in the adiabatic tunneling regime.
- The PPT model demonstrated applicability across various ionization regimes.
- Ionization pathways for molecular hydrogen were determined using different pump laser wavelengths (800, 400, 267 nm).
Conclusions:
- The developed interferometer offers high sensitivity for plasma density diagnostics.
- Experimental results provide insights into the validity of ADK and PPT models for laser-driven ionization.
- The study elucidates ionization mechanisms in noble gases and molecular hydrogen under varying laser conditions.
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