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Highly ordered laser imprinted plasmonic metasurfaces for polarization sensitive perfect absorption.

Anna C Tasolamprou1, Evangelos Skoulas2, George Perrakis2

  • 1Institute of Electronic Structure and Laser, Foundation for Research and Technology Hellas, N. Plastira 100, Crete, 71110, Heraklion, Greece. atasolam@iesl.foth.gr.

Scientific Reports
|November 17, 2022
PubMed
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We developed novel polarization-sensitive plasmonic metasurfaces using pulsed laser technology. These metasurfaces enable tunable polarization control and high extinction ratios for near- and mid-infrared light.

Area of Science:

  • Plasmonics
  • Metamaterials
  • Nanotechnology

Background:

  • Surface plasmon resonance (SPR) is crucial for optical sensing and manipulation.
  • Existing fabrication methods for plasmonic metasurfaces can be complex and costly.
  • Developing versatile and direct fabrication techniques is essential for advancing metasurface applications.

Purpose of the Study:

  • To present a novel, direct fabrication method for polarization-sensitive gap surface plasmon metasurfaces using pulsed laser light.
  • To demonstrate the tunability of polarization control by varying the insulating cavity's size and material.
  • To achieve high extinction ratios for polarization control in the near- and mid-infrared spectral regions.

Main Methods:

  • Fabrication of metasurfaces via laser-induced periodic surface structures on nanometer-thick nickel (Ni) films.

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  • Construction of a metal-insulator-metal (MIM) structure with TiO2 and ZnO dielectric layers, followed by gold (Au) evaporation.
  • Characterization using Fourier-transform infrared (FTIR) spectroscopy to analyze resonant absorption and polarization sensitivity.
  • Main Results:

    • Successful creation of metal-insulator-metal plasmonic metasurfaces with highly-ordered, sinusoidal metallic nanowires.
    • Demonstration of sharp, resonant gap surface plasmons enabling polarization control in reflection.
    • Observation of polarization-sensitive perfect absorption and high extinction ratios in the near- and mid-IR.
    • Experimental validation of well-defined, controllable, and sharp resonances with polarization-sensitive absorption response.

    Conclusions:

    • Pulsed laser direct material processing offers a versatile alternative for fabricating advanced plasmonic metasurfaces.
    • The developed metasurfaces exhibit significant polarization control capabilities, tunable via the insulating cavity.
    • These findings pave the way for novel optical devices with tailored polarization responses in the infrared spectrum.