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Updated: Aug 17, 2025

Gradient Echo Quantum Memory in Warm Atomic Vapor
Published on: November 11, 2013
Molecular orientation echoes via concerted terahertz and near-IR excitations
Abstract:
A new and efficient method for orientation echo spectroscopy is presented and realized experimentally. The excitation scheme utilizes concerted rotational excitations by both ultrashort terahertz and near-IR pulses and its all-optical detection is enabled by the molecular orientation-induced second harmonic method [J. Phys. Chem. A126, 3732 (2022)10.1021/acs.jpca.2c03237]. This method provides practical means for orientation echo spectroscopy of gas phase molecules and highlights the intriguing underlying physics of coherent rotational dynamics induced by judiciously-orchestrated interactions with both resonant (terahertz) and nonresonant (NIR) fields.
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