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Interface Engineering of All-Solid-State Batteries Based on Inorganic Solid Electrolytes.

Lei Xi1, Dechao Zhang1, Xijun Xu1

  • 1Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials School of Materials Science and Engineering, South China University of Technology, Guangzhou, 510641, P. R. China.

Chemsuschem
|January 19, 2023
PubMed
Summary
This summary is machine-generated.

All-solid-state batteries (ASSBs) offer higher energy density and safety but face interface challenges. This study explores interface modification strategies to improve contact and stability for better ASSB performance.

Keywords:
all-solid-state batteriesinorganic solid electrolyteinterfacemodificationstack pressure

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) are promising for next-generation energy storage due to high energy density and safety.
  • Poor solid-solid contact and limited chemical/electrochemical stability at interfaces hinder ASSB performance, increasing resistance.
  • Interface issues lead to contact failure and degeneration during cycling, impacting coulombic efficiency and battery lifespan.

Purpose of the Study:

  • To provide a fundamental understanding of physical contact and chemical/electrochemical properties of ASSB interfaces.
  • To summarize recent advancements in interface modification techniques for inorganic solid electrolytes (SEs).
  • To highlight strategies for enhancing the performance and stability of ASSBs.

Main Methods:

  • Review and analysis of interface modification strategies for inorganic SEs in ASSBs.
  • Discussion of methods including SE doping, morphology optimization, and interlayer/coating introduction.
  • Examination of compatible electrode materials and the role of applied stack pressure during cycling.

Main Results:

  • Identified key interface modification techniques to prevent side reactions at cathode/anode-SE interfaces.
  • Emphasized the importance of maintaining constant extra stack pressure for optimal electrochemical performance.
  • Detailed understanding of how interface engineering impacts coulombic efficiency and cycling stability.

Conclusions:

  • Interface modification is crucial for overcoming the limitations of inorganic SEs in ASSBs.
  • Strategies like doping, coatings, and optimized electrode materials effectively improve interface contact and stability.
  • Future research should focus on these interface engineering approaches for practical, high-performance ASSBs.