A new approach of air pollution regionalization based on geographically weighted variations for multi-pollutants in...

Air pollution regionalization is a key and necessary action to identify pollution regions for implementing control measures. Here we present a new approach called Geographically Weighted Rotation Empirical Orthogonal Function (GWREOF) for air pollution regionalization in China. Compared with previous methods, such as EOF, REOF, and K-mean, GWREOF better accounts for the variability of air pollution conditions driven by emission patterns and meteorology with centralized spatial locations. We apply GWREOF to multiple air pollutants (such as PM_2.5, O₃, and other monitored air pollutants) and air quality metrics using their measured spatial and temporal variations in 337 Chinese cities over 2015-2020. We find that the regionalization results for different air pollutants are highly similar, primarily determined by topography and meteorological conditions in China. Therefore, we propose an integrated regionalization result, which identifies 18 air pollution control regions in China and can be applied to multiple pollutants and different years. We further analyze PM_2.5, O₃, and O_X (O₃ + NO₂) pollution levels and their correlations in these regions. PM_2.5 and O₃ correlations are generally strongly positive in southern China while negative in northern China. However, PM_2.5 and O_X correlations are broadly positive in China, reflecting the crucial role of atmospheric oxidizing capacity. Regional-specific and coordinated control measures are in need as China's air pollution strategy transits from PM_2.5-focused to PM_2.5-O₃ synergic control.