Dynamical Axions in U(1) Quantum Spin Liquids

Since their proposal nearly half a century ago, physicists have sought axions in both high energy and condensed matter settings. Despite intense and growing efforts, to date, experimental success has been limited, with the most prominent results arising in the context of topological insulators. Here, we propose a novel mechanism whereby axions can be realized in quantum spin liquids. We discuss the necessary symmetry requirements and identify possible experimental realizations in candidate pyrochlore materials. In this context, the axions couple to both the external and the emergent electromagnetic fields. We show that the interaction between the axion and the emergent photon leads to a characteristic dynamical response, which can be measured experimentally in inelastic neutron scattering. This Letter sets the stage for studying axion electrodynamics in the highly tunable setting of frustrated magnets.