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X-ray Crystallography02:18

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The size of the unit cell and the arrangement of atoms in a crystal may be determined from measurements of the diffraction of X-rays by the crystal, termed X-ray crystallography.
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Diffraction is the change in the direction of travel experienced by an electromagnetic wave when it encounters a physical barrier whose dimensions are comparable to those of the wavelength of the light. X-rays are electromagnetic radiation with wavelengths about as long as the distance between neighboring...
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Resonant inelastic x-ray scattering data for Ruddlesden-Popper and reduced Ruddlesden-Popper nickelates.

G Fabbris1,2, D Meyers3,4, Y Shen3

  • 1Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York, 11973, USA. gfabbris@anl.gov.

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|March 29, 2023
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Summary
This summary is machine-generated.

We present open resonant inelastic x-ray scattering (RIXS) data for Ruddlesden-Popper nickelates La₄Ni₃O₁₀ and La₄Ni₃O₈. This data aims to resolve inconsistencies and facilitate comparisons with cuprates.

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Solid State Chemistry

Background:

  • Ruddlesden-Popper and reduced Ruddlesden-Popper nickelates are explored as potential analogues to high-temperature superconducting cuprates.
  • The extent of similarity between these nickelate and cuprate materials remains a significant point of scientific discussion.
  • Resonant inelastic x-ray scattering (RIXS) is a key technique for investigating their electronic and magnetic excitations.

Purpose of the Study:

  • To address inconsistencies in previous RIXS studies on nickelates.
  • To provide a standardized, open dataset for La₄Ni₃O₁₀ and La₄Ni₃O₈.
  • To enable detailed comparative analysis between nickelates and cuprates.

Main Methods:

  • Utilized resonant inelastic x-ray scattering (RIXS) spectroscopy.
  • Collected and curated open RIXS data for specific nickelate compounds.
  • Focused on La₄Ni₃O₁₀ and La₄Ni₃O₈ samples.

Main Results:

  • Successfully generated and shared open RIXS data for La₄Ni₃O₁₀ and La₄Ni₃O₈.
  • The presented data serves as a benchmark for future studies.
  • Facilitates direct comparison of excitation spectra.

Conclusions:

  • The open data release is expected to mitigate sample-dependent inconsistencies in RIXS studies.
  • This resource will advance the understanding of nickelate-cuprate relationships.
  • Promotes collaborative research in the field of correlated electron systems.