A Versatile Method for Synthesis of Light-Activated, Magnet-Steerable Organic-Inorganic Hybrid Active Colloids

The immense potential of active colloids in practical applications and fundamental research calls for an efficient method to synthesize active colloids of high uniformity. Herein, a facile method is reported to synthesize uniform organic-inorganic hybrid active colloids based on the wetting effect of polystyrene (PS) with photoresponsive inorganic nanoparticles in a tetrahydrofuran/water mixture. The results show that a range of dimer active colloids can be produced by using different inorganic components, such as AgCl, ZnO, TiO₂, and Fe₂O₃ nanoparticles. Moreover, the strategy provides a simple way to prepare dual-drive active colloids by a rational selection of the starting organic materials, such as magnetic PS particles that result in light and magnet dual-drive active colloids. The motions of these active colloids are quantified, and well-controlled movements are demonstrated.