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Perovskite single-crystal thin films: preparation, surface engineering, and application.

Zemin Zhang1, Wooyeon Kim2, Min Jae Ko3

  • 1Institute of Photoelectronic Thin Film Devices and Technology, Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin, Engineering Research Center of Thin Film Optoelectronics Technology (MoE), Nankai University, Tianjin, 300350, China.

Nano Convergence
|May 22, 2023
PubMed
Summary

Large-area perovskite single-crystal thin films (SCTFs) offer high performance for optoelectronics. This review details preparation methods, surface engineering, and applications, addressing commercialization challenges.

Keywords:
Crystal growthLight-emitting devicePerovskitePhotodetectorPhotovoltaicSingle crystalSurface engineering

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Area of Science:

  • Materials Science
  • Optoelectronics
  • Nanotechnology

Background:

  • Perovskite single-crystal thin films (SCTFs) are crucial for optoelectronic devices due to low defect density, long carrier diffusion length, and stability.
  • Challenges remain in large-area, high-throughput preparation, surface defect reduction, and device manufacturing.

Purpose of the Study:

  • To review advances in large-area, high-quality perovskite SCTFs.
  • To analyze nucleation and crystallization mechanisms and preparation methods.
  • To discuss surface engineering, applications, and commercialization.

Main Methods:

  • Analysis of nucleation and crystallization mechanisms.
  • Classification of perovskite SCTF preparation methods.
  • Review of surface engineering techniques.

Main Results:

  • Progress in controlling area, thickness, and quality of perovskite SCTFs.
  • Overview of surface engineering strategies.
  • Summary of applications in photovoltaics, photodetectors, LEDs, artificial synapses, and transistors.

Conclusions:

  • Perovskite SCTFs show great promise for advanced optoelectronic devices.
  • Further research is needed to overcome challenges in large-scale manufacturing and commercialization.