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High-Thermal-Conductivity and High-Fluidity Heat Transfer Emulsion with 89 wt % Suspended Liquid Metal Microdroplets
Suyeon Kim1, Seongeun Kang1, Joohyung Lee1
1Department of Chemical Engineering, Myongji University, 116 Myongji-ro, Cheoin-gu, Yongin, Gyeonggi-do 17058, Korea.
ACS Omega
|May 30, 2023
Summary
Researchers developed advanced heat transfer fluids using liquid metal microdroplets in oil. These emulsions significantly boost thermal conductivity while maintaining excellent fluidity for efficient thermal energy transfer.
Area of Science:
- Materials Science
- Fluid Dynamics
- Heat Transfer
Background:
- Colloidal suspensions with conductive particles enhance heat transfer fluids.
- High particle concentrations are limited by fluid vitrification.
- Liquid metal (LM) offers high thermal conductivity (k).
Purpose of the Study:
- To create a high thermal conductivity and high fluidity heat transfer fluid.
- To investigate eutectic Ga-In liquid metal as a soft filler in paraffin oil.
- To evaluate emulsion production methods for optimal performance.
Main Methods:
- Dispersing eutectic Ga-In liquid metal microdroplets in paraffin oil.
- Producing emulsions using probe-sonication and rotor-stator homogenization (RSH).
- Measuring thermal conductivity and viscosity at high filler loadings (up to 50 vol %).
Main Results:
- Significant thermal conductivity enhancement (Δk ~409% with probe-sonication, ~261% with RSH) at 50 vol % LM.
- Heat transport improved via high-k LM fillers above the percolation threshold.
- RSH-produced emulsion maintained high fluidity with low viscosity increase and no yield stress.
Conclusions:
- Emulsion-type heat transfer fluids with liquid metal offer superior thermal conductivity and fluidity.
- RSH method is effective for producing stable, high-performance heat transfer fluids.
- These fluids show potential for diverse thermal energy transfer applications.

