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Related Experiment Video

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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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PEO-Based Solid Composite Polymer Electrolyte for High Capacity Retention All-Solid-State Lithium Metal Battery.

Kashif Khan1,2, Muhammad Bilal Hanif3, Hu Xin2

  • 1Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China, Huzhou, Zhejiang, 313001, P. R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|September 15, 2023
PubMed
Summary

This study enhances poly(ethylene oxide) solid polymer electrolytes with hybrid fillers for high-energy lithium metal batteries. The new electrolytes show improved conductivity and stability, enabling long-lasting battery performance.

Keywords:
all-solid-state lithium metal batterieshybrid fillersionic conductivitypolyethylene oxidesolid polymer electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Science

Background:

  • Poly(ethylene oxide) (PEO) solid polymer electrolytes (SPEs) offer limited ionic conductivity and electrochemical stability for high-energy lithium metal batteries.
  • Garnet-type Li6.4 La3 Zr1.4 Ta0.6 O12 (LLZTO) is a promising filler but suffers from high interfacial resistance in PEO SPEs.

Purpose of the Study:

  • To develop a novel hybrid filler-designed SPE for improved lithium metal battery performance.
  • To overcome the limitations of PEO and LLZTO in achieving high ionic conductivity and electrochemical stability.

Main Methods:

  • Fabrication of a solid composite membrane incorporating hybrid fillers into a PEO-based SPE.
  • Electrochemical characterization including ionic conductivity, Li+ transference number, and cycling stability tests.
  • Assembly and testing of Li/Li symmetric cells and LiFePO4/Li batteries.

Main Results:

  • Achieved a maximum ionic conductivity of 1.9 × 10-4 S cm-1 and a Li+ transference number of 0.67 at 40 °C.
  • Demonstrated stable cycling for 2000 h in Li/Li symmetric cells at 0.1 mA cm-2.
  • Delivered a high-rate capacity of 159.2 mAh g-1 at 1 C with 95.2% retention after 400 cycles in LiFePO4/Li batteries.

Conclusions:

  • A hybrid filler strategy effectively enhances the electrochemical performance of PEO-based SPEs.
  • The developed SPEs are suitable for high-performance all-solid-state lithium metal batteries.
  • This approach offers a viable pathway for advancing next-generation energy storage solutions.