Enhanced second harmonic generation from a quasi-periodic silver dendritic metasurface

The preparation of the vast majority of nonlinear optical metal metasurfaces currently relies on complex top-down methods such as electron beam or ion beam etching, which are expensive and difficult to meet the requirement of large area preparation. In this paper, an easily prepared quasi-periodic silver dendritic metasurface model with highQfactor is established in the near-infrared band based on a simple and easy-to-operate electrochemical deposition method. The simulations prove that the silver dendritic metasurface has a highQfactor (exceeds 10⁴) because of its strong electric field localization ability, which is analogous to the superposition of multiple split-ring resonators. It is demonstrated that the second harmonic generation (SHG) intensity of the dendritic metasurface at a large incident angle (such as 85°) is about 30 times that of the metasurface at a small incident angle when thex-polarized pump light is incident obliquely to break the centrosymmetry of the metasurface. The influences of the incident angle or dendritic structure's dimensions on theQfactor and SHG efficiency have also been researched through a lot of simulation. This easily prepared quasi-periodic silver dendritic metasurface SHG device may provide a new avenue for the development and application of miniature, integratable nonlinear optical devices.