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Precursor Engineering of Solution-Processed Sb2 S3 Solar Cells.

Yanyan Li1, Ruiming Li1, Zhenglin Jia1

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Small (Weinheim an Der Bergstrasse, Germany)
|October 24, 2023
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Summary

Introducing silver (Ag) ions into antimony sulfide (Sb2S3) sol-gel precursors significantly enhances thin film solar cell performance. This method achieves a record 7.73% power conversion efficiency, offering a promising route for solution-processed photovoltaics.

Keywords:
AgSbS2Sb2S3chalcogenidescharge transportsolar cells

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Area of Science:

  • Materials Science
  • Renewable Energy
  • Photovoltaics

Background:

  • Antimony-based chalcogenides, particularly antimony sulfide (Sb2S3) thin films, show promise for next-generation solar cells.
  • Sb2S3 offers facile fabrication, simple composition, good charge transport, and stability.
  • Current efficient Sb2S3 solar cells often rely on time-consuming solution-based methods like chemical bath deposition and hydrothermal techniques.

Purpose of the Study:

  • To investigate the effect of incorporating silver (Ag) ions into Sb2S3 sol-gel precursors.
  • To enhance the crystallization and charge transport properties of Sb2S3 thin films.
  • To develop a more efficient and potentially faster fabrication method for Sb2S3-based solar cells.

Main Methods:

  • Incorporation of silver (Ag) ions into antimony sulfide (Sb2S3) sol-gel precursors.
  • Fabrication of Ag-incorporated Sb2S3 thin films for photovoltaic applications.
  • Characterization of structural, electrical, and photovoltaic properties of the fabricated solar cells.

Main Results:

  • Silver ion incorporation modulated Sb2S3 crystallization and charge transport.
  • Enhanced crystallinity and increased charge carrier mobility were observed in Ag-modified Sb2S3.
  • Ag-incorporated Sb2S3 solar cells showed improved fill factor and open-circuit voltage, reducing recombination losses.
  • The champion solar cell achieved a record power conversion efficiency of 7.73% with antireflection coating.

Conclusions:

  • Silver ion incorporation is an effective strategy to improve the performance of Sb2S3 thin film solar cells.
  • This approach offers a viable alternative to traditional methods, paving the way for efficient solution-processed photovoltaics.
  • The achieved efficiency is comparable to state-of-the-art Sb2S3 solar cells fabricated using chemical bath deposition and hydrothermal techniques.