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Photodiode-based time zero determination for ultrafast electron microscopy.

S T Kempers1, S Borrelli1, E R Kieft2

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Structural Dynamics (Melville, N.Y.)
|November 9, 2023
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Summary
This summary is machine-generated.

We developed a simple photodiode method to precisely measure time zero in ultrafast electron microscopy. This technique ensures accurate temporal overlap of electron and laser pulses for pump-probe experiments.

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Area of Science:

  • Ultrafast electron microscopy
  • Femtosecond laser physics
  • Materials science

Background:

  • Pump-probe experiments in ultrafast electron microscopy (UEM) demand precise temporal overlap between excitation (pump) and probing (probe) pulses.
  • Accurate determination of time zero (t0) is critical for resolving ultrafast dynamics in materials.
  • Existing methods for t0 determination can be complex or costly.

Purpose of the Study:

  • To present a cost-effective and user-friendly photodiode-based method for measuring time zero in UEM.
  • To enable precise temporal alignment of single-electron pulses with femtosecond laser pulses.
  • To establish a foundation for achieving micrometer and picosecond spatiotemporal resolution.

Main Methods:

  • Development of a photodiode integrated into a sample holder for UEM.
  • Utilizing the photodiode to detect the temporal overlap between electron and laser pulses.
  • Characterization of the temporal resolution of the developed alignment method.

Main Results:

  • A photodiode-based alignment device was successfully implemented for time zero measurements.
  • The initial device achieved a temporal resolution of 24 picoseconds (ps).
  • The photodiode's design was identified as the limiting factor for temporal resolution.

Conclusions:

  • The photodiode method offers a practical approach for achieving time zero alignment in UEM.
  • Future improvements using photodiodes with lower capacitance will enhance temporal and spatial resolution.
  • This technique paves the way for advanced spatiotemporal investigations in UEM.