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High-time resolution PM2.5 source apportionment assisted by spectrum-based characteristics analysis.

Jie Liu1, Fangjingxin Ma2, Tse-Lun Chen3

  • 1School of Water Conservancy & Civil Engineering, Northeast Agricultural University, Harbin 150030, China; Institute of Environmental Engineering (IfU), ETH Zürich, 8093 Zürich, Switzerland.

The Science of the Total Environment
|December 6, 2023
PubMed
Summary

This study introduces a new framework for analyzing particulate matter (PM2.5) pollution by combining spectral analysis with source apportionment. The findings reveal secondary inorganic aerosols as the primary contributor to Beijing

Keywords:
High-time resolutionPM(2.5) pollutionSource apportionmentSpectral analysisSpectrum characteristics extraction

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Area of Science:

  • Environmental Science
  • Atmospheric Chemistry
  • Data Analysis

Background:

  • Particulate matter (PM2.5) pollution requires effective source apportionment for effective mitigation strategies.
  • Frequency spectrum analysis offers potential for extracting characteristics of PM2.5 pollution events.

Purpose of the Study:

  • To develop and apply an integrated framework for PM2.5 source apportionment using spectral analysis and receptor modeling.
  • To extract spectrum characteristics of PM2.5 pollution anomalies for improved source identification.

Main Methods:

  • Combined Fast Fourier Transform (FFT) and Continuous Wavelet Transform (CWT) for spectral analysis.
  • Utilized Positive Matrix Factorization (PMF) receptor model for source contribution assessment.
  • Applied the framework to hourly PM2.5 data from Beijing during the winter heating period.

Main Results:

  • Successfully captured spectrum characteristics (frequency, location, duration, intensity) of PM2.5 pollution anomalies.
  • Identified secondary inorganic aerosols as the dominant PM2.5 source (50.59%) during Beijing's winter heating period.
  • Quantified contributions from other sources: biomass burning (15.01%), vehicle emissions (11.00%), coal combustion (10.70%), road dust (5.31%), industrial processes (3.88%), and fireworks (3.51%).

Conclusions:

  • The integrated spectral analysis and PMF framework provides robust insights into PM2.5 pollution dynamics.
  • This approach enhances understanding of temporal evolution, source identification, and contribution quantification of PM2.5.