Related Experiment Video
Updated: Jul 9, 2025

Experimental Methods for Spin- and Angle-Resolved Photoemission Spectroscopy Combined with Polarization-Variable Laser
Published on: June 28, 2018
An improved source of spin-polarized electrons based on spin exchange in optically pumped rubidium vapor
K J Ahrendsen1, K W Trantham2, D Tupa3
1Jorgensen Hall, University of Nebraska, Lincoln, Nebraska 68588-0299, USA.
Abstract:
We have improved a polarized electron source in which unpolarized electrons undergo collisions with a mixture of buffer gas molecules and optically spin-polarized Rb atoms. With a nitrogen buffer gas, the source reliably provides spin polarization between 15% and 25% with beam currents >4 μA. Vacuum pump upgrades mitigate problems caused by denatured diffusion pump oil, leading to longer run times. A new differential pumping scheme allows the use of higher buffer gas pressures up to 800 mTorr. With a new optics layout, the Rb polarization is continuously monitored by a probe laser and improved pump laser power provides more constant high polarization. We have implemented an einzel lens to better control the energy of the electrons delivered to the target chamber and to preferentially select electron populations of higher polarization. The source is designed for studies of biologically relevant chiral molecule samples, which can poison photoemission-based GaAs polarized electron sources at very low partial pressures. It operates adjacent to a target chamber that rises to pressures as high as 10-4 Torr and has been implemented in a first experiment with chiral cysteine targets.
Related Concept Videos
Atomic Nuclei: Nuclear Relaxation Processes
Atomic Nuclei: Nuclear Spin State Overview
Spin–Spin Coupling: Two-Bond Coupling (Geminal Coupling)
The central atom need not be NMR-active because its electrons are affected by the electron polarization of the spin-active atoms. However, spin information is transmitted less effectively than in one-bond coupling, and 2J values are usually weaker than 1J values. The energy of...
Double Resonance Techniques: Overview
Spin decoupling is usually achieved by...
Nuclear Overhauser Enhancement (NOE)
Atomic Nuclei: Magnetic Resonance

