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Updated: Jul 2, 2025

Experimental Methods for Spin- and Angle-Resolved Photoemission Spectroscopy Combined with Polarization-Variable Laser
Published on: June 28, 2018
Nonlinear spin-orbit coupling in optical thin films
Domenico de Ceglia1,2, Laure Coudrat3, Iännis Roland4
1CNIT and Department of Information Engineering, University of Brescia, Via Branze, 38, Brescia, 25123, Italy. domenico.deceglia@unibs.it.
Abstract:
Tunable generation of vortex beams holds relevance in various fields, including communications and sensing. In this paper, we demonstrate the feasibility of nonlinear spin-orbit interactions in thin films of materials with second-order nonlinear susceptibility. Remarkably, the nonlinear tensor can mix the longitudinal and transverse components of the pump field. We observe experimentally our theoretical predictions in the process of second-harmonic generation from a thin film of aluminum gallium arsenide, a material platform widely spread for its role in the advancement of active, nonlinear, and quantum photonic devices. In particular, we prove that a nonlinear thin film can be used to produce vector vortex beams of second-harmonic light when excited by circularly-polarized Gaussian beams.
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