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Regenerative Solid Interfaces Enhance High-Performance All-Solid-State Lithium Batteries.

Zhaoxin Yu1, Yaobin Xu2, Michael Kindle1

  • 1Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, United States.

ACS Nano
|April 24, 2024
PubMed
Summary

Researchers developed a regenerative solid interface using nanosized lithium iodide to stabilize lithium metal anodes in all-solid-state lithium batteries. This breakthrough enhances battery performance and longevity, enabling over 1000 hours of stable operation.

Keywords:
all-solid-state batteryhalogenlithiumlithium−sulfur batterysolid-state electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium batteries (ASSLBs) face challenges with lithium anode interfacial instability.
  • Dynamic changes during lithium plating/stripping cause performance degradation.

Purpose of the Study:

  • To create a conductive and regenerative solid interface for ASSLBs.
  • To enhance lithium anode stability and improve overall cell performance.

Main Methods:

  • In situ generation of nanosized lithium iodide (nano-LiI) from the solid-state electrolyte.
  • Utilizing the reversible diffusion of nano-LiI during lithium plating and stripping.
  • Directly using metallic lithium as the anode.

Main Results:

  • Achieved stable operation of metallic lithium anode for over 1000 hours at high current densities and elevated temperatures.
  • Demonstrated stable cycling of all-solid-state lithium-sulfur batteries for over 250 cycles.
  • Improved adhesion and Li+ transport between the lithium anode and solid-state electrolyte.

Conclusions:

  • The regenerative nano-LiI interface effectively tackles solid interfacial challenges in ASSLBs.
  • This approach facilitates uniform lithium plating/stripping and enhances battery longevity.
  • Offers insights for designing advanced interfaces for high-performance ASSLBs.