Field-Induced Rocking-Curve Effects in Attosecond Electron Diffraction

Recent advances in electron microscopy trigger the question of whether attosecond electron diffraction can resolve atomic-scale electron dynamics in crystalline materials in space and time. Here, we explore the ultrafast dynamics of the relevant electron-lattice scattering process. We drive a single-crystalline silicon membrane with the optical cycles of near-infrared laser light and use phase-locked attosecond electron pulses to produce electron diffraction patterns as a function of delay. For all Bragg spots, we observe time-dependent intensity changes and position shifts that are correlated with a time shift of 0.5-1.2  fs. For single-cycle excitation pulses with strong peak intensity, the correlations become nonlinear. The origins of these effects are local and integrated beam deflections by the optical electric and magnetic fields at the crystal membrane. Those deflections modify the diffraction intensities in addition to the atomic structure factor dynamics by time-dependent rocking-curve effects. However, the measured time delays and symmetries allow one to disentangle both effects. Future attosecond electron diffraction and microscopy experiments need to be based on these results.