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    Area of Science:

    • Optics and Photonics
    • Spectroscopy
    • Materials Science

    Background:

    • Converting terahertz (THz) signals to the optical domain is crucial for advancing THz sensing and spectroscopy.
    • Four-wave mixing (FWM) is a nonlinear optical process that can be used for frequency conversion.

    Purpose of the Study:

    • To investigate the conversion of intense broadband THz pulses into the optical domain.
    • To explore the application of THz-four-wave mixing (FWM) in nonlinear optical processes.
    • To demonstrate resonant amplification of THz-FWM signals in fluoride crystals.

    Main Methods:

    • Mixing intense broadband THz pulses (central frequency ΩTHz) with an optical pump (ωp).
    • Observing the generated optical signal at ωs = 2(ωp - Δωp) - ΩTHz, where Δωp accounts for pump spectral broadening.
    • Utilizing calcium fluoride (CaF2), barium fluoride (BaF2), and magnesium fluoride (MgF2) as nonlinear media.

    Main Results:

    • A THz-four-wave mixing (FWM) signal was observed near 400 nm.
    • The signal generation was attributed to resonantly amplified FWM.
    • Efficient conversion was demonstrated in CaF2, BaF2, and MgF2 crystals.

    Conclusions:

    • THz-FWM is a viable method for converting THz signals to the optical domain.
    • Resonant amplification significantly enhances the THz-FWM signal.
    • Fluoride crystals are effective media for THz-to-optical conversion, paving the way for novel THz applications.