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All-electronic Nanosecond-resolved Scanning Tunneling Microscopy: Facilitating the Investigation of Single Dopant Charge Dynamics
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High dynamic range scanning tunneling microscopy.

Ajla Karić1, Carolina A Marques1, Berk Zengin1

  • 1Department of Physics, University of Zurich, Winterthurerstrasse 190, Zurich CH-8057, Switzerland.

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|August 6, 2024
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Summary
This summary is machine-generated.

We enhance scanning tunneling microscope (STM) dynamic range by actively removing current harmonics. This method prevents preamplifier saturation, enabling high-fidelity spectroscopy and imaging without hardware modification.

Keywords:
Active power FilterAmplifier saturationBand-structureDensity of statesDynamic rangeHigh Dynamic Range Scanning Tunneling MicroscopyScanning tunneling microscopyScanning tunneling spectroscopy

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Area of Science:

  • Physics
  • Materials Science
  • Nanotechnology

Background:

  • Scanning tunneling microscopy (STM) is crucial for nanoscale imaging and spectroscopy.
  • Nonlinearities in current-voltage characteristics generate current harmonics.
  • These harmonics can saturate preamplifiers, limiting the dynamic range of STM measurements, especially at low impedances or high gains.

Purpose of the Study:

  • To increase the dynamical range of a scanning tunneling microscope (STM).
  • To overcome preamplifier saturation issues caused by current harmonics.
  • To enable high dynamic range spectroscopy and imaging in STM.

Main Methods:

  • Actively subtracting dominant current-harmonics generated by nonlinearities.
  • Utilizing the phase relationship between excitation voltage and current-harmonics for cancellation.
  • Employing a compensating capacitor at the preamplifier input to cancel harmonics via displacement current.
  • Using two phase-synchronized voltage sources and a multi-frequency lock-in amplifier.

Main Results:

  • Successful cancellation of dominant current-harmonics.
  • Prevention of current preamplifier saturation.
  • Demonstration that DC current removal has no effect and first harmonic removal causes a reversible shift in differential conductance.
  • Achieved high dynamic range spectroscopy and imaging.

Conclusions:

  • The developed method effectively expands the dynamic range of STM.
  • Active harmonic subtraction is a viable technique for improving STM performance.
  • The approach requires minimal hardware changes, relying on synchronized voltage sources and lock-in amplification.