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Updated: Jun 11, 2025

Synthesis and Performance Characterizations of Transition Metal Single Atom Catalyst for Electrochemical CO2 Reduction
Published on: April 10, 2018
A universal strategy for the synthesis of transition metal single atom catalysts toward electrochemical CO2 reduction
Bowen Li1, Yan Liang2, Yinlong Zhu1
1Institute for Frontier Science, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, China. zhuyl1989@nuaa.edu.cn.
Abstract:
Herein, a pyrolysis-induced precursor transformation strategy has been proposed. Using pre-synthesized PDA-M as a precursor, the production of transition metal single atom catalysts (SACs) has been achieved, with compositional flexibility at high metal loadings. In particular, the Ni SAC sample has shown promising CO selectivity when evaluated for the electrochemical CO2 reduction reaction, reaching 29.8 mA cm-2 CO partial current density and 90.3% CO faradaic efficiency at -1.05 V vs. RHE.
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