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Two-Dimensional MoSi2N4 Family: Progress and Perspectives Form Theory
Wenyuan Jin1, Jingning Zuo2, Jiafei Pang3,4
1Institute of Physics, Henan Academy of Sciences, Zhengzhou 450046, China.
Abstract:
Recently, a new two-dimensional (2D) layered MoSi2N4 has been successfully synthesized by chemical vapor deposition without knowing the 3D counterparts [ Science 2020, 369, 670-674]. The unique septuple-atomic-layer structure and diverse composition of MoSi2N4 have drawn tremendous interest in studying 2D MA2Z4 systems based on the MoSi2N4 structure. As an emerging family of 2D materials, MA2Z4 materials exhibit a wide range of properties and excellent tunability, making them highly promising for various applications. Herein, we summarize recent significant progress in property characterization of the MA2Z4 family. The electronic, magnetic, thermal transport, and superconducting properties, including their tunability through strain engineering and elemental substitution, are presented and elaborated in detail. Further perspectives and new opportunities of the emerging MA2Z4 family are presented at the end of this Perspective.
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