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Porous PDMS-ZnO Wearable Gas Sensor for Acetone Biomarker Detection and Breath Analysis.
Yanru Chen1, Yixin Liu1, Jiaqi Liu1
1Shenzhen Intern ational Graduate School, Tsinghua University, Shenzhen 518055, China.
ACS Applied Materials & Interfaces
|October 31, 2024
Summary
This study introduces a wearable UV-assisted gas sensor for nonintrusive breath acetone detection. The flexible sensor demonstrates stable and accurate health monitoring, even under mechanical strain and varying humidity.
Area of Science:
- Materials Science
- Nanotechnology
- Wearable Technology
Background:
- Growing demand for global health monitoring necessitates nonintrusive detection methods.
- Breath acetone (BrAce) analysis offers a noninvasive approach to health assessment.
- Development of flexible and robust sensors is crucial for wearable applications.
Purpose of the Study:
- To develop a compact, conformal wearable UV-assisted gas-sensing system for breath acetone detection.
- To analyze breath events and concentrations using a flexible sensor.
- To investigate the synergistic effects of UV irradiation and porous structure on sensor performance.
Main Methods:
- Fabrication of an intrinsically flexible porous polydimethylsiloxane (PDMS)-zinc oxide (ZnO) composite layer (PPZL).
- Utilizing ultraviolet (UV) irradiation to enhance gas-sensing properties.
- Testing sensor performance under mechanical strain (bending, tensile) and varying humidity.
Main Results:
- The UV-assisted wearable sensor reliably detects BrAce concentrations from 1 to 100 ppm at room temperature.
- The sensor maintains stable performance over 20 days with <5% signal degradation, even under mechanical strain.
- Accurate analysis of breathing patterns and BrAce concentrations was achieved, with consistent response under up to 70% relative humidity.
Conclusions:
- The developed flexible acetone gas sensor provides a portable solution for health management.
- The synergistic effect of UV and porous structure enhances acetone response and mechanical robustness.
- The fabrication method offers a pathway for designing flexible metal oxide gas sensors.

