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Excitonic Hamiltonians for Calculating Optical Absorption Spectra and Optoelectronic Properties of Molecular Aggregates and Solids
Published on: May 27, 2020
General theory of cavity-mediated interactions between low-energy matter excitations
Carlos J Sánchez Martínez1,2, Frieder Lindel1,2, Francisco J García-Vidal1,2
1Departamento de Física Teórica de la Materia Condensada, Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
Abstract:
The manipulation of low-energy matter properties such as superconductivity, ferromagnetism, and ferroelectricity via cavity quantum electrodynamics engineering has been suggested as a way to enhance these many-body collective phenomena. In this work, we investigate the effective interactions between low-energy matter excitations induced by the off-resonant coupling with cavity electromagnetic modes. We extend a previous work by going beyond the dipole approximation accounting for the full polarization and magnetization densities of matter. We further include the often neglected diamagnetic interaction and, for the cavity, we consider general linear absorbing media with possibly non-local and non-reciprocal response. We demonstrate that, even in this general scenario, the effective cavity-induced interactions between the matter degrees of freedom are of electrostatic and magnetostatic nature. This confirms the necessity of a multimode description for cavity engineering of matter systems where the low-energy assumption holds. Our findings provide a theoretical framework for studying the influence of general optical environments on extended low-energy matter excitations.
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