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Optimization studies on output stabilization time and graphene oxide concentration in graphene-based flexible
Sangeetha Gopan G S1,2, Nelsa Abraham2,3, Harikrishnan R S4
1Department of ECE, College of Engineering Trivandrum, Thiruvananthapuram, Kerala 695016, India.
Flexible laser-induced graphene micro-supercapacitors (MSCs) were fabricated using graphene oxide (GO) coated polyimide. The study optimized GO concentration and found capacitance stabilized after six days, showing potential for wearable electronics.
Area of Science:
- Materials Science
- Nanotechnology
- Electrochemistry
Background:
- Miniature energy storage is crucial for flexible and wearable electronics.
- Micro-supercapacitors (MSCs) offer a promising solution for compact energy storage.
Purpose of the Study:
- To fabricate flexible laser-induced graphene-based MSCs.
- To optimize graphene oxide (GO) concentration for enhanced performance.
- To evaluate the stability and durability of the MSCs.
Main Methods:
- Laser-induced graphene fabrication on GO-coated polyimide film.
- Assembly of MSCs with H2SO4/polyvinyl alcohol (PVA) gel electrolyte.
- Daily capacitance assessment over ten days and electrochemical impedance spectroscopy.
Main Results:
- Capacitance stabilized after six days of assessment.
- Optimal GO concentration yielded an areal capacitance of 10.07 mF cm-2 at 13 µA cm-2.
- The optimized MSC retained 87.9% capacitance after 5000 cycles and showed reliable performance under bending.
Conclusions:
- Flexible laser-induced graphene MSCs are viable for energy storage in wearable devices.
- Optimized GO concentration and stability are key for practical applications.
- The developed MSCs demonstrate excellent durability and flexibility for self-powered systems.
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